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Table of contents
Spectroscopy and microscopy experiments confirmed the successful in situ synthesis of C-dots within the PSiO 2 nanostructure host and showed that the C-dots retained their unique fluorescence properties while being embedded within the PSiO 2 pores. The potential of this hybrid system for modulating the photophysical properties of both components and for sensing applications is significant.
The integration of PSiO 2 and C-dots enhances the sensing performance of these optically responsive materials in comparison with the individual components. Importantly, the C-dots embedded within the PSiO 2 matrix exhibited a higher sensitivity than the solubilized C-dots, attesting to the significance of the nanoporous environment in promoting interactions between the carbon nanoparticles and adsorbed analytes and highlighting a useful strategy for enhancing the sensing capabilities of C-dots. Moreover, it should be emphasized that the hybrid allowed for real-time sensitive detection of small molecules, which is one of the main limitations of reflectivity-based PSi sensors.
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We are currently exploring several approaches for enhancing the sensitivity and selectivity of the reported hybrids, including the use of capture probes and changing the PSiO 2 matrix from a single porous layer to a multilayered structure. Thus, the proof-of-concept work presented here provides a generic sensing platform that can potentially be applied to the rapid detection and identification of a variety of analytes.
Baker, S. Luminescent carbon nanodots: emergent nanolights. Lim, S. Carbon quantum dots and their applications. Zhu, S. Highly photoluminescent carbon dots for multicolor patterning, sensors, and bioimaging. Bhunia, S. Imaging cancer cells expressing the folate receptor with carbon dots produced from folic acid. Chembiochem 17 , — Ding, C.
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Functional surface engineering of C-dots for fluorescent biosensing and in vivo bioimaging. Sun, X. Fluorescent carbon dots and their sensing applications. Trends Anal. Nanoscale 8 , — Dong, Y. Sensing applications of luminescent carbon based dots. Analyst , — Graphene quantum dot as a green and facile sensor for free chlorine in drinking water. Polyamine-functionalized carbon quantum dots as fluorescent probes for selective and sensitive detection of copper ions.
Nanomaterials applications
Lin, X. Encapsulation of strongly fluorescent carbon quantum dots in metal—organic frameworks for enhancing chemical sensing. Wang, R. Carbon quantum dot-functionalized aerogels for NO2 gas sensing. Anglin, E. Porous silicon in drug delivery devices and materials. Drug Deliv. Kilian, K. The importance of surface chemistry in mesoporous materials: lessons from porous silicon biosensors.
Chen, M.
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Electric-Field-assisted protein transport, capture, and interferometric sensing in carbonized porous silicon films. Massad-Ivanir, N. Rodriguez, G. Real-time detection of small and large molecules using a porous silicon grating-coupled bloch surface wave label-free biosensor. SPIE 27 , Weiss, S. Current status and outlook for silicon-based optical biosensors.
E 41 , — Guan, B. Mesoporous silicon photonic crystal microparticles: towards single-cell optical biosensors. Faraday Discuss. Mariani, S. ACS Sensors 1 , — Vilensky, R. Oxidized porous silicon nanostructures enabling electrokinetic transport for enhanced DNA detection. Zhang, H.
Porous silicon optical microcavity biosensor on silicon-on-insulator wafer for sensitive DNA detection. Biosensors Bioelectron. Gaur, G.
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Immobilization of quantum dots in nanostructured porous silicon films: characterizations and signal amplification for dual-mode optical biosensing. Jiao, Y. Dual-mode sensing platform based on colloidal gold functionalized porous silicon. Krismastuti, F. Porous silicon resonant microcavity biosensor for matrix metalloproteinase detection. Liu, C.
Enhancement of QDs' fluorescence based on porous silicon Bragg mirror. B , — Urmann, K. Label-free optical biosensors based on aptamer-functionalized porous silicon scaffolds. Sailor, M. Pacholski, C. Biosensing using porous silicon double-layer interferometers: reflective interferometric Fourier transform spectroscopy. Reflective interferometric fourier transform spectroscopy: a self-compensating label-free immunosensor using double-layers of porous SiO2. Wang, Y. Carbon quantum dots: synthesis, properties and applications. C 2 , — Sa'ar, A. Photoluminescence from silicon nanostructures: the mutual role of quantum confinement and surface chemistry.
Hydrogels synthesized in electrochemically machined porous Si hosts: effect of nano-scale confinement on polymer properties. Soft Matter 8 , — Boubaya, M. Butler, J. Low-voltage scanning electron-microscopy of polymer. Polymer 36 , — Hirota, M. The role of trypsin, trypsin inhibitor, and trypsin receptor in the onset and aggravation of pancreatitis.
Yamashita, K. A tumor-suppressive role for trypsin in human cancer progression. Cancer Res. Zhang, X. Photoelectrochemical biosensor for detection of adenosine triphosphate in the extracts of cancer cells.
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Zhou, Z. Ouyang, H. Quantitative analysis of the sensitivity of porous silicon optical biosensors.